The hit featuring Rihanna had already been nominated for song of the year and his "Recovery" was also nominated for album of the year.
Other song of the year nominees up for record of the year included Cee Lo's "(Expletive) You" and Lady Antebellum's "Need You Now."
Also nominated was Jay-Z and Alicia Keys' anthem for New York, "Empire State of Mind"; and "Nothin' On You" by rapper B.o.B and featuring Bruno Mars.
The announcement was made as part of the Grammys' hourlong live nominations special on CBS from Club Nokia in Los Angeles.
The Grammys will be awarded Sunday, Feb. 13, at Staples Center in Los Angeles and broadcast live on CBS.